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• W2316283057 startingPage "5639" @default.
• W2316283057 abstract "Understanding charge transfer reactions between quantum dots (QD) and metal oxides is fundamental for improving photocatalytic, photovoltaic, and electronic devices. The complexity of these processes makes it difficult to find an optimum QD size with rapid charge injection and low recombination. We combine time-domain density functional theory with nonadiabatic molecular dynamics to investigate the size and temperature dependence of the experimentally studied electron transfer and charge recombination at CdSe QD–TiO2 nanobelt (NB) interfaces. The electron injection rate shows strong dependence on the QD size, increasing for small QDs. The rate exhibits Arrhenius temperature dependence, with the activation energy of the order of millielectronvolts. The charge recombination process occurs due to coupling of the electronic subsystem to vibrational modes of the TiO2 NB. Inelastic electron–phonon scattering happens on a picosecond time scale, with strong dependence on the QD size. Our simulations demonstrate t..." @default.
• W2316283057 created "2016-06-24" @default.
• W2316283057 creator A5025610159 @default.
• W2316283057 creator A5061633372 @default.
• W2316283057 date "2015-03-03" @default.
• W2316283057 modified "2023-09-27" @default.
• W2316283057 title "Size and Temperature Dependence of Electron Transfer between CdSe Quantum Dots and a TiO₂ Nanobelt" @default.
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• W2316283057 doi "https://doi.org/10.1021/jp5110278" @default.
• W2316283057 hasPublicationYear "2015" @default.
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