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• W2316303601 abstract "Thermally assembled hydrogen bonding cages which are neither size nor guest specific have been developed using a poly (vinyl alcohol) (PVA) host. A water-soluble conjugated polymer poly(2,5-bis(3-sulfonatopropoxy)-1,4-phenylene, disodium salt-alt-1,4-phenylene) (PPP-OPSO${}_{3}$) as a donor and tris(2,2-bipyridyl)- ruthenium(II) [Ru(bpy)${}_{3}$${}^{2+}$] as an acceptor have been isolated and trapped in such a PVA matrix network. This is a unique system that shows negligible exciton diffusion and the donor and acceptor predominantly interact by a direct single step excitation transfer process (DSSET). Singlet and triplet exciton quenching have been studied. Time-resolved fluorescence lifetime measurement at different acceptor concentrations has enabled us to determine the dimensionality of the energy-transfer process within the PVA scaffold. Our results reveal that the PVA hydrogen bonding network effectively isolates the donor-acceptor molecules in a two-dimensional layer structure (lamella) leading to the condition where a precise control of the energy and charge transfer is possible." @default.
• W2316303601 created "2016-06-24" @default.
• W2316303601 creator A5028216232 @default.
• W2316303601 creator A5058497622 @default.
• W2316303601 date "2012-12-13" @default.
• W2316303601 modified "2023-10-02" @default.
• W2316303601 title "Controlled energy transfer between isolated donor-acceptor molecules intercalated in thermally self-ensemble two-dimensional hydrogen bonding cages" @default.
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• W2316303601 doi "https://doi.org/10.1103/physrevb.86.235420" @default.
• W2316303601 hasPublicationYear "2012" @default.
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