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• W2316387515 endingPage "373" @default.
• W2316387515 startingPage "367" @default.
• W2316387515 abstract "A series of (Gd2−xLix)Ti2O7−x with x = 0.050–0.150, abbreviated as GLT-2L were prepared by the addition of 2x mole of LiO0.5 self-flux in the parent compound. Preparation temperatures were between 1450 and 1500°C depending on the amount of the self-flux addition. Relative densities of all GLT-2L samples were larger than 97.9(3)%. However, the parent compound, Gd2Ti2O7 has no LiO0.5 co-existence, it has a relative density of 92.8(4)% only, although it was prepared at a higher temperature, 1650°C. Among the GLT-2L samples, the one with x = 0.110 has the highest total electrical conductivity, 6.17(6) × 10−5 S·cm−1 at 700°C and the lowest activation energy, 0.95(3) eV. Doping Li+ ions into the Gd-site of Gd2Ti2O7, preparation temperature was lowered and samples become denser. Meanwhile, vacancies were created and electrical conductivity was increased. At 500°C, average ionic transference numbers (ti) found for all samples are fully ionic. Increasing temperature, ti decreases slightly due to the increase of the fractional electronic conductivity of the (Gd2−xLix)Ti2O7−x, which is a mixed conductor at high temperature. Ti atoms are in the the mixed valence states." @default.
• W2316387515 created "2016-06-24" @default.
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• W2316387515 date "2015-01-01" @default.
• W2316387515 modified "2023-10-14" @default.
• W2316387515 title "Electrical properties of the (Gd_2&minus;<i>_x</i>Li<i>_x</i>)Ti₂O_7&minus;<i>_x</i> co-existence with the LiO_0.5 self-flux" @default.
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• W2316387515 doi "https://doi.org/10.2109/jcersj2.123.367" @default.
• W2316387515 hasPublicationYear "2015" @default.
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