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• W2316388596 abstract "Infrared emission following the photolysis of SO2 by a 193 nm laser pulse (20 ns duration) was recorded with 500 ns time and 10 cm–1 spectral resolution. Spectral analyses of the time-resolved spectra revealed the vibrationally excited nascent SO population distribution as (v = 1)/(v = 2)/(v = 3)/(v = 4)/(v = 5) = 0.54 ± 0.04, 1.00 ± 0.03, 0.00 ± 0.03, 0.01 ± 0.03, and 0.10 ± 0.03. The nascent SO was found to be rotationally excited with an average rotational temperature around 1000 K for v = 1 and v = 2 levels and 300 K for the v = 5 level. The vibrationally excited SO likely originates from two distinct dissociation mechanisms; the v = 1 and 2 populations are generated through intersystem crossing between the C̃ state and a repulsive state (23A′), and the v = 5 population is generated through internal conversion from the C̃ to the X̃ state. Efficient V–V energy transfer from nascent vibrationally excited SO to SO2(ν1) is also observed. The appearance of the SO2(ν1) ν1 = 2 emission, before that from the ν1 = 1 population is consistent with the previous report that the Δν = −2 channel is more efficient than the Δν = −1 channel." @default.
• W2316388596 created "2016-06-24" @default.
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• W2316388596 date "2011-12-12" @default.
• W2316388596 modified "2023-10-18" @default.
• W2316388596 title "Photolysis (193 nm) of SO₂: Nascent Product Energy Distribution Examined through IR Emission" @default.
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• W2316388596 doi "https://doi.org/10.1021/jp2061943" @default.
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