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- W2316456912 abstract "Fischer-Tropsch synthesis, i.e., the catalytic conversion of syngas (CO + H2) into hydrocarbons, is a key step for the indirect transformation of non-petroleum carbon resources such as coal, methane, and biomass into liquid fuels and chemicals. The products follow the Anderson-Schulz-Flory distribution over conventional Fischer-Tropsch catalysts, which is unselective for particular products. The design and preparation of highly selective Fischer-Tropsch catalysts and the realization of selectivity control for C–C coupling are the most challenging targets in the modern C<sub>1</sub> chemistry. This review outlines recent advances in the theoretical studies on C–C coupling mechanism on the surfaces of typical Fischer-Tropsch catalysts, and briefly summarizes the key factors affecting the product selectivity in Fischer-Tropsch synthesis with emphases on recent studies on the effects of the size and the microenvironment of active metal particles. This paper also highlights recent developments of bifunctional Fischer-Tropsch catalytic systems capable of catalyzing not only the hydrogenation of CO to heavy hydrocarbons but also the hydrocracking/ isomerization of heavy hydrocarbons. A new strategy for tuning the Fischer-Tropsch product selectivity by controlling the secondary reactions has been proposed." @default.
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- W2316456912 date "2012-03-01" @default.
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- W2316456912 title "Selectivity tuning for the hydrogenation of carbon monoxide into hydrocarbons" @default.
- W2316456912 doi "https://doi.org/10.1360/032011-749" @default.
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