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• W2316572293 abstract "The stoichiometric rare-earth compound ${mathrm{YbInCu}}_{4}$ is known for its first-order valence transition at ${T}_{a}ensuremath{approx}55mathrm{K}$ and ambient pressure. Although this valence transition has been extensively studied by various volume-sensitive experimental methods, highly surface-sensitive photoemission measurements in the vuv energy range [ultraviolet photoemission spectroscopy (UPS)] could not observe a sharp valence change of the Yb valence ${v}_{mathrm{Yb}}$ at the transition temperature. Instead there is only a smooth temperature dependence of ${v}_{mathrm{Yb}}$ over a large temperature range. Furthermore, the low-temperature values for the hole-occupation number ${n}_{h}{=v}_{mathrm{Yb}}ensuremath{-}2$ from UPS are significantly below the values of volume-sensitive measurements. Here we present temperature-dependent photoemission data on ${mathrm{YbInCu}}_{4}$ measured at photon energies of $hensuremath{nu}=1486mathrm{eV}$ [x-ray photoemission spectroscopy (XPS)] with a significantly increased information depth in comparison to previous experiments with lower photon energies. These data clearly show the existence of a valence transition at the extended sampling depth of the XPS experiment, in contrast to results from the distorted near-surface region." @default.
• W2316572293 created "2016-06-24" @default.
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• W2316572293 date "2001-04-27" @default.
• W2316572293 modified "2023-09-25" @default.
• W2316572293 title "Reply to “Comment on ‘Photoemission experiments on<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>YbInCu</mml:mi></mml:mrow><mml:mrow><mml:mn>4</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mo>:</mml:mo></mml:math>Surface effects and temperature dependence’ ”" @default.
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• W2316572293 doi "https://doi.org/10.1103/physrevb.63.197102" @default.
• W2316572293 hasPublicationYear "2001" @default.
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