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- W2316603964 abstract "We derive the class of population balance equations (PBE), recently applied to model the Viedma deracemization experiment, from an underlying microreversible kinetic reaction scheme. The continuum limit establishing the relationship between the micro- and macroscopic processes and the associated particle fluxes erases the microreversible nature of the molecular interactions in the population growth rate functions and limits the scope of such PBE models to strict kinetic control. The irreversible binary agglomeration processes modeled in those PBEs contribute an additional source of kinetic control. These limitations are crucial regarding the question of the origin of biological homochirality, where the interest in any model lies precisely in its ability for absolute asymmetric synthesis and the amplification of the tiny inherent statistical chiral fluctuations about the ideal racemic composition up to observable enantiometric excess levels." @default.
- W2316603964 created "2016-06-24" @default.
- W2316603964 creator A5032885365 @default.
- W2316603964 creator A5037097673 @default.
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- W2316603964 date "2015-02-02" @default.
- W2316603964 modified "2023-09-26" @default.
- W2316603964 title "Modeling spontaneous chiral symmetry breaking and deracemization phenomena: Discrete versus continuum approaches" @default.
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- W2316603964 doi "https://doi.org/10.1103/physreve.91.022801" @default.
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