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• W2316951396 startingPage "4032" @default.
• W2316951396 abstract "The dense ceramic membranes BaCo(0.7)Fe(0.2)Nb(0.1)O(3-δ) (BCFN) combined with GdBaCo(2-x)Fe(x)O(5+δ) (0 ≤ x ≤ 2.0) surface modification layers was investigated for hydrogen production by partial oxidation reforming of coke oven gas (COG). As oxygen permeation of BCFN membrane is controlled by the rate surface exchange kinetics, the GdBaCo(2-x)Fe(x)O(5+δ) materials improve the oxygen permeation flux of the BCFN membrane by 20-44% under helium atmosphere at 750 °C. The maximum oxygen permeation flux reached 14.4 mL min(-1) cm(-2) in the GdBaCoFeO(5+δ) coated BCFN membrane reactor at 850 °C, and a CH(4) conversion of 94.9%, a H(2) selectivity of 88.9%, and a CO selectivity of 99.6% have been achieved. The GdBaCo(2-x)Fe(x)O(5+δ) coating materials possess uniform porous structure, fast oxygen desorption rate and good compatibility with the membrane, which showed a potential application for the surface modification of the membrane reactor." @default.
• W2316951396 created "2016-06-24" @default.
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• W2316951396 date "2011-09-30" @default.
• W2316951396 modified "2023-10-01" @default.
• W2316951396 title "Enhancing the Oxygen Permeability of BaCo_0.7Fe_0.2Nb_0.1O_3−δ Membranes by Coating GdBaCo_2-<i>x</i>Fe_<i>x</i>O_5+δ for Partial Oxidation of Coke Oven Gas to Syngas" @default.
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• W2316951396 doi "https://doi.org/10.1021/am200892b" @default.
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