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• W2316967609 abstract "A-site-ordered perovskite-structure oxides with Mn and V at A′ and B sites, respectively, were synthesized by using a high-pressure method. Valence-state analyses revealed that the A-site substitution modulated the valence states of the Mn ions at the A′ site and V ions at the B site sequentially. By changing the A-site ions from Na+ to Ca2+ and from Ca2+ to La3+, the valence distribution changed site-selectively from Na+Mn2.33+3V4+4O12 to Ca2+Mn2+3V4+4O12 and to La3+Mn2+3V3.75+4O12. The electrons of the A′-site Mn were localized and contributed to the magnetic properties, that is, spin-glass-like behavior in NaMn3V4O12 and antiferromagnetic behavior in CaMn3V4O12 and LaMn3V4O12. The valence electrons of the B-site V, in contrast, were delocalized, as could be seen from the low resistivity of the samples. The delocalized electrons at the B-site V did not correlate with the localized spins at the A′-site Mn." @default.
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• W2316967609 date "2012-11-02" @default.
• W2316967609 modified "2023-10-01" @default.
• W2316967609 title "Site-Selective Doping Effect in AMn₃V₄O₁₂ (A = Na⁺, Ca²⁺, and La³⁺)" @default.
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• W2316967609 doi "https://doi.org/10.1021/ja308851f" @default.
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