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- W2316971231 abstract "A rigid rod-like organic molecular ensemble comprised of a triarylamine electron donor, a 2,2′-bipyridine (bpy) ligand, and a 9,10-anthraquinone acceptor was synthesized and reacted with suitable metal precursors to yield triads with Ru(bpy)32+, Os(bpy)32+, and [Ir(2-(p-tolyl)pyridine)2(bpy)]+ photosensitizers. Photoexcitation of these triads leads to long-lived charge-separated states (τ = 80–1300 ns) containing a triarylamine cation and an anthraquinone anion, as observed by transient absorption spectroscopy. From a combined electrochemical and optical spectroscopic study, the thermodynamics and kinetics for the individual photoinduced charge-separation and thermal charge-recombination events were determined; in some cases, measurements on suitable donor–sensitizer or sensitizer–acceptor dyads were necessary. In the case of the ruthenium and iridium triads, the fully charge-separated state is formed in nearly quantitative yield." @default.
- W2316971231 created "2016-06-24" @default.
- W2316971231 creator A5000683714 @default.
- W2316971231 creator A5024442454 @default.
- W2316971231 creator A5056952888 @default.
- W2316971231 creator A5058688452 @default.
- W2316971231 date "2012-05-23" @default.
- W2316971231 modified "2023-09-27" @default.
- W2316971231 title "Photoinduced Electron Transfer in Linear Triarylamine–Photosensitizer–Anthraquinone Triads with Ruthenium(II), Osmium(II), and Iridium(III)" @default.
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- W2316971231 doi "https://doi.org/10.1021/ic300558s" @default.
- W2316971231 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22621319" @default.
- W2316971231 hasPublicationYear "2012" @default.
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