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• W2317261343 abstract "Pressure-induced amorphization of methane hydrate has been investigated by molecular dynamics simulation. In accord with experimental results of Tulk et al., a crystalline ensuremath{rightarrow} amorphous transition was confirmed at 3.3 GPa where the water lattice collapsed around the encaged methane. Thermal annealing at 5.5 GPa allows the water to adopt a lower energy conformation with a denser structure. In both structures, methane molecules are immobilized and maintain long-range correlation as in the crystal. Consequently, both phases are predicted to revert back to the crystalline form upon decompression. Pressure-induced amorphization is a nonequilibrium process due to a mechanical instability; the interconversion between kinetically stable amorphous phases is a relaxation effect." @default.
• W2317261343 created "2016-06-24" @default.
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• W2317261343 date "2012-09-18" @default.
• W2317261343 modified "2023-09-26" @default.
• W2317261343 title "Pressure-induced amorphization of methane hydrate" @default.
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• W2317261343 doi "https://doi.org/10.1103/physrevb.86.104109" @default.
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