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- W2317395148 endingPage "19675" @default.
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- W2317395148 abstract "In supramolecular polymers, directional interactions control the constituting units connectivity, but dispersion forces may conspire to make complex organizations. Here we report on the long-range order and order–disorder transition (ODT) of main-chain supramolecular polymers based on poly(propylene oxide) (PPO) spacers functionalized on both ends with thymine. Below the ODT temperature (TODT), these compounds are semicrystalline with a lamellar structure, showing nanophase separation between crystallized thymine planes and amorphous PPO layers. Above TODT, they are amorphous and homogeneous even though their X-ray scattering spectrum reveals a peak. This peak is due to correlation hole effect resulting from contrast between end-functional groups and spacer. Macroscopically, the transition is accompanied by dramatic flow and mechanical properties changes." @default.
- W2317395148 created "2016-06-24" @default.
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- W2317395148 date "2011-11-17" @default.
- W2317395148 modified "2023-09-25" @default.
- W2317395148 title "Order–Disorder Transition in Supramolecular Polymers" @default.
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- W2317395148 doi "https://doi.org/10.1021/ja209126a" @default.
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