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- W2317895989 abstract "We present density functional theory calculations of carrier multiplication properties in a system of strongly coupled silicon nanocrystals. Our results suggest that nanocrystal-nanocrystal interaction can lead to a reduction of the carrier multiplication energy threshold without altering the carrier multiplication efficiency at high energies, in agreement with experiments. The time evolution of the number of electron-hole pairs generated in a system of strongly interacting nanocrystals upon absorption of high-energy photons is analyzed by solving a system of coupled rate equations, where exciton recycling mechanisms are implemented. We reconsider the role played by Auger recombination which is here accounted also as an active, nondetrimental process." @default.
- W2317895989 created "2016-06-24" @default.
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- W2317895989 date "2014-08-19" @default.
- W2317895989 modified "2023-09-23" @default.
- W2317895989 title "Red-Shifted Carrier Multiplication Energy Threshold and Exciton Recycling Mechanisms in Strongly Interacting Silicon Nanocrystals" @default.
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- W2317895989 doi "https://doi.org/10.1021/ja5057328" @default.
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