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• W2317925580 endingPage "13044" @default.
• W2317925580 startingPage "13040" @default.
• W2317925580 abstract "Reactions of oxygen-chemisorbed cobalt and iron cluster cations (Co(n)O(m)(+) and Fe(n)O(m)(+); n = 3-6, m = 1-3) with an NH(3) molecule have been investigated in comparison with their bare metal cluster cations at a collision energy of 0.2 eV by use of a guided ion beam tandem mass spectrometer. We have observed three kinds of reaction products, which come from NH(3) chemisorption with and without release of a metal atom from the cluster and dehydrogenation of the chemisorbed NH(3). Reaction cross sections and branching fractions are strongly influenced by the number of oxygen atoms introduced onto the metal clusters. Oxygen-chemisorbed metal clusters with particular compositions such as Co(4)O(+), Co(5)O(2)(+), and Fe(5)O(2)(+) are extremely reactive for NH(3) dehydrogenation, whereas Co(4)O(2)(+) and Fe(4)O(2)(+) exhibit high reactivity for NH(3) chemisorption with metal release. The enhancement of dehydrogenation for specific compositions can be interpreted in terms of competition between O-H and neighboring Co-H (or Fe-H) formation." @default.
• W2317925580 created "2016-06-24" @default.
• W2317925580 creator A5015881305 @default.
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• W2317925580 date "2010-11-19" @default.
• W2317925580 modified "2023-09-27" @default.
• W2317925580 title "Enhancement of Ammonia Dehydrogenation by Introduction of Oxygen onto Cobalt and Iron Cluster Cations" @default.
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• W2317925580 doi "https://doi.org/10.1021/jp109118d" @default.
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