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• W2318040319 startingPage "60" @default.
• W2318040319 abstract "The hydrogenation of aromatics under mild conditions remains a challenge in the fields of synthetic and petroleum chemistry. Described herein is a new catalytic material that shows excellent catalytic performance in terms of activity, selectivity, and reusability in the hydrogenation of aromatics in solvent-free systems under mild conditions. The catalyst, consisting of rhodium nanoparticles supported on nanocrystalline hydroxyapatite, can quantitatively hydrogenate neat benzene to cyclohexane with exceptionally high rates (initial TOF > 10(3) h(-1)) at 298 K and 3 bars of initial H(2) pressure. This new material maintains its inherent catalytic activity after several reuses. Importantly, catalyst preparation does not require elaborate procedures because the active metal nanoparticles are readily formed from the in situ reduction of Rh(3+)-exchanged hydroxyapatite while submerged in the aromatic solvent at room temperature under 3 bars of H(2) pressure." @default.
• W2318040319 created "2016-06-24" @default.
• W2318040319 creator A5016487357 @default.
• W2318040319 creator A5048885361 @default.
• W2318040319 creator A5075500520 @default.
• W2318040319 date "2011-12-19" @default.
• W2318040319 modified "2023-10-18" @default.
• W2318040319 title "Rhodium(0) Nanoparticles Supported on Nanocrystalline Hydroxyapatite: Highly Effective Catalytic System for the Solvent-Free Hydrogenation of Aromatics at Room Temperature" @default.
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• W2318040319 doi "https://doi.org/10.1021/la2044174" @default.
• W2318040319 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22145782" @default.
• W2318040319 hasPublicationYear "2011" @default.
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