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• W2318082103 startingPage "9601" @default.
• W2318082103 abstract "In recent years, supramolecular organization of thiophene derivatives, oligo- and polythiophene, have been developed with various designs to achieve complex functions. Here, we describe the synthesis and characterization of a conjugated polymer with thymidine side chain bases and polythiophene backbones (PTT) instead of phosphate bonds in DNA, and the PTT exhibits exceptional fluorescence quenching efficiency upon binding of Cu2+ ions in aqueous medium, which is suggested to be electron transfer from the π* orbit at the excited state of PTT to the 3d orbit of Cu2+ ions and subsequent Cu2+-mediated interpolymer π-stacking aggregation. Furthermore, Cu2+ ions can be selectively and easily monitored by the fluorescence quenching of PTT, which can be used for detection of Cu2+ ions with good selectivity and high sensitivity in aqueous medium. Both experimental and theoretical methods have been devoted to demonstrate the strong affinity and steric interaction of PTT toward Cu2+. These findings will illustrate new directions for the design of nucleobase-functionalized materials with transition metals responsive activity." @default.
• W2318082103 created "2016-06-24" @default.
• W2318082103 creator A5024425081 @default.
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• W2318082103 creator A5080303772 @default.
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• W2318082103 date "2014-06-12" @default.
• W2318082103 modified "2023-09-27" @default.
• W2318082103 title "Nucleobase-Functionalized Conjugated Polymer for Detection of Copper(II)" @default.
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• W2318082103 doi "https://doi.org/10.1021/am502978w" @default.
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• W2318082103 hasPublicationYear "2014" @default.
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