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• W2318150963 abstract "Single-particle characterization of Antarctic aerosols was performed to investigate the impact of marine biogenic sulfur species on the chemical compositions of sea-salt aerosols in the polar atmosphere. Quantitative energy-dispersive electron probe X-ray microanalysis was used to characterize 2900 individual particles in 10 sets of aerosol samples collected between March 12 and 16, 2009 at King Sejong Station, a Korean scientific research station located at King George Island in the Antarctic. Two size modes of particles, i.e., PM2.5–10 and PM1.0–2.5, were analyzed, and four types of particles were identified, with sulfur-containing sea-salt particles being the most abundant, followed by genuine sea-salt particles without sulfur species, iron-containing particles, and other species including CaCO3/CaMg(CO3)2, organic carbon, and aluminosilicates. When a sulfur-containing sea-salt particle showed an atomic concentration ratio of sulfur to sodium of >0.083 (seawater ratio), it is regarded as containing nonsea-salt sulfate (nss-SO42–) and/or methanesulfonate (CH3SO3–), which was supported by attenuated total reflection Fourier transform-infrared imaging measurements. These internal mixture particles of sea-salt/CH3SO3–/SO42– were very frequently encountered. As nitrate-containing particles were not encountered, and the air-masses for all of the samples originated from the Pacific Ocean (based on 5-day backward trajectories), the oxidation of dimethylsulfide (DMS) emitted from phytoplanktons in the ocean is most likely to be responsible for the formation of the mixed sea-salt/CH3SO3–/SO42– particles." @default.
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• W2318150963 date "2011-07-08" @default.
• W2318150963 modified "2023-10-16" @default.
• W2318150963 title "Single-Particle Characterization of Summertime Antarctic Aerosols Collected at King George Island Using Quantitative Energy-Dispersive Electron Probe X-ray Microanalysis and Attenuated Total Reflection Fourier Transform-Infrared Imaging Techniques" @default.
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• W2318150963 doi "https://doi.org/10.1021/es200936m" @default.
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• W2318150963 hasPublicationYear "2011" @default.
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