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• W2318303905 abstract "The nonradiative dark channels in the L-edge fluorescence spectra from transition-metal aqueous solution identify the ultrafast charge-transfer processes playing an important role in many biological and chemical systems. Yet, the exact origin of such spectral dips with respect to the X-ray transmission spectrum has remained unclear. In the present study we explore the nature of the underlying decay mechanism of 2p core-excited Co2+ in water by probing the nonradiative Auger-type electron emission channel using photoelectron spectroscopy from a liquid microjet. Our measurements demonstrate unequivocally that metal-to-water charge transfer quenches fluorescence and will inevitably lead to a dip in the total-fluorescence-yield X-ray absorption spectrum. This is directly revealed from the resonant enhancement of valence signal intensity arising from the interference of two identical final states created by a direct and Auger-electron emission, respectively." @default.
• W2318303905 created "2016-06-24" @default.
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• W2318303905 date "2012-01-12" @default.
• W2318303905 modified "2023-09-25" @default.
• W2318303905 title "Origin of Dark-Channel X-ray Fluorescence from Transition-Metal Ions in Water" @default.
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• W2318303905 doi "https://doi.org/10.1021/ja207931r" @default.
• W2318303905 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22175947" @default.
• W2318303905 hasPublicationYear "2012" @default.
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