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• W2318338049 abstract "Elucidating the effect of porous host on the intrinsic physicochemical properties and reactivity of the encapsulated nanosized hydrous ferric oxides (HFOs) is believed important to better understand how HFOs interact with ionic pollutants inside the pore region. Here we prepared a hybrid adsorbent (HFO–CMPS) by dispersing nanosized HFOs onto an inactive porous polymeric support (i.e., chloromethylated polystyrene, CMPS). A surface complexation model (SCM) was employed to quantitatively evaluate the acid–base reactions and adsorption behaviors of HFO–CMPS as compared to the bare HFOs. Results demonstrated that the intrinsic equilibrium constants for acid–base reactions of surface sites of HFOs distinctly changed upon loading, that is, the log K(+) values decreased, while its log K(−) values increased, resulting in its pHpzc value shifting from ∼8.2 to ∼6.3. Meanwhile, the titration curves of HFO–CMPS showed a markedly weaker dependence upon ionic strength. The results of model fittings of Cu(II) and As(V) ..." @default.
• W2318338049 created "2016-06-24" @default.
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• W2318338049 date "2013-03-19" @default.
• W2318338049 modified "2023-09-27" @default.
• W2318338049 title "Surface Chemistry of Nanosized Hydrated Ferric Oxide Encapsulated Inside Porous Polymer: Modeling and Experimental Studies" @default.
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• W2318338049 doi "https://doi.org/10.1021/jp3119154" @default.
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