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• W2318371911 startingPage "14738" @default.
• W2318371911 abstract "We report the crystallization of a subsitutionally doped organic conductor based on a host lattice composed of spiro-bis(phenalenyl)boron radicals. Co-crystallization of solutions of spiro-bis(9-oxidophenalenone)boron radical [PLY(O,O)]2B mixed with selected amounts of spiro-bis(9-oxidophenalenone)beryllium [PLY(O,O)]2Be leads to the formation of a series of solid-state solutions of composition [PLY(O,O)]2B(1–x)Bex. The dopant molecules [PLY(O,O)]2Be serve to introduce holes into the lattice of spins provided by the [PLY(O,O)]2B radicals and lead to a systematic increase in the conductivity while decreasing the activation energy of the conduction process and leaving the solid-state structure relatively unperturbed. While the energies of the hole sites are expected to be high, the results are consistent with the interpretation of the electronic structure of [PLY(O,O)]2B in terms of the resonating valence bond model." @default.
• W2318371911 created "2016-06-24" @default.
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• W2318371911 date "2014-10-08" @default.
• W2318371911 modified "2023-10-18" @default.
• W2318371911 title "Enhanced Electrical Conductivity in a Substitutionally Doped Spiro-bis(phenalenyl)boron Radical Molecular Solid" @default.
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• W2318371911 doi "https://doi.org/10.1021/ja508903z" @default.
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• W2318371911 hasPublicationYear "2014" @default.
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