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- W2318532077 abstract "A new series of strongly greenish-blue to blue emitting Cu(NN)(POP)+ (POP = bis[2-(dipenylphosphino)phenyl]ether) complexes containing N-linked 2-pyridyl pyrazolate diimine ligands [Cu(pypz)(POP)]BF4 (1), [Cu(pympz)(POP)]BF4 (2), and [Cu(pytfmpz)(POP)]BF4 (3) (pypz = 1-(2-pyridyl)pyrazole, pympz = 3-methyl-1-(2-pyridyl)pyrazole, and pytfmpz = 3-trifluoromethyl-1-(2-pyridyl)pyrazole) have been designed and synthesized. Their structural, electrochemical, and photophysical properties have been characterized. The complexes 1–3 exhibit high photoluminescence quantum yields (PLQYs) at room temperature both in nitrogen-saturated CH2Cl2 (up to 45%) and in neat solid (up to 87%), which are comparable to the reported highest values for the cuprous complexes. The temperature dependence of spectroscopic properties and emission decay behaviors reveal the presence of two thermally equilibrated emitting states. At temperatures below 150 K, the lowest triplet state (T1) is the predominant emitting state resulting in the ..." @default.
- W2318532077 created "2016-06-24" @default.
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- W2318532077 date "2013-09-18" @default.
- W2318532077 modified "2023-10-17" @default.
- W2318532077 title "Rational Design of Strongly Blue-Emitting Cuprous Complexes with Thermally Activated Delayed Fluorescence and Application in Solution-Processed OLEDs" @default.
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- W2318532077 doi "https://doi.org/10.1021/cm4024309" @default.
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