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• W2318562237 startingPage "2104" @default.
• W2318562237 abstract "A series of triarylimidazoles was synthesized and characterized electrochemically. The synthetic route is general, providing a pathway to 30 redox mediators that exhibit a > 700 mV range of accessible potentials. Most of the triarylimidazoles display three oxidation peaks where the first redox couple is quasi-reversible. The electronic character of the substituents affects the oxidation potential. This is exemplified by a linear correlation between the first oxidation potential and the sum of the Hammett σ+ substituent constants, as well as with a series of calculated ionization potentials. We close by putting forward a rule of thumb stating that for a given mediator, the upper limit of accessible potentials can be extended by at least 500 mV beyond the largest recorded value. A rationale, the conditions under which the rule is likely to apply, and an example are provided." @default.
• W2318562237 created "2016-06-24" @default.
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• W2318562237 date "2012-12-11" @default.
• W2318562237 modified "2023-10-04" @default.
• W2318562237 title "Triarylimidazole Redox Catalysts: Electrochemical Analysis and Empirical Correlations" @default.
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• W2318562237 doi "https://doi.org/10.1021/jo302309m" @default.
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