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- W2318565360 abstract "We report the synthesis, morphology, and optoelectronic device applications of novel biaxially extended quaterthiophene– (4T−) and octithiophene– (8T−) vinylene conjugated polymers, P4TV and P8TV, synthesized via Stille coupling reactions. P4TV and P8TV exhibited smaller energy band gaps of 1.69 and 1.78 eV than that of parent polythiophenes, respectively, due to the reduced conformation distortion by the vinylene linkage. The HOMO energy levels of P4TV and P8TV were −5.02 and −5.13 eV, respectively, resulting in air stable device performance. The highest field effect hole mobilities of P4TV and P8TV were 0.12 and 0.0018 cm2 V–1 s–1, respectively, with on/off ratios around 104–105. The higher carrier mobility of P4TV was related to its ordered structure as evidenced from the TEM, AFM, and grazing incidence X-ray diffraction results. The power conversion efficiency (PCE) of the P4TV/ PC71BM based photovoltaic cells (PV) under the illumination of AM 1.5G (100 mW/cm2) was 4.04%, which was significantly highe..." @default.
- W2318565360 created "2016-06-24" @default.
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- W2318565360 date "2012-03-26" @default.
- W2318565360 modified "2023-10-16" @default.
- W2318565360 title "Biaxially Extended Quaterthiophene– and Octithiophene–Vinylene Conjugated Polymers for High Performance Field Effect Transistors and Photovoltaic Cells" @default.
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- W2318565360 doi "https://doi.org/10.1021/ma300313y" @default.
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