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• W2318631608 abstract "Nowadays molecular nanoporous networks have numerous uses in surface nanopatterning applications and in studies of host-guest interactions. Trimesic acid (TMA), a benzene derivative with three carboxylic groups, is a marvelous building block for forming 2D H-bonded porous networks. Here, we report a low-temperature study of the nanoporous chicken-wire superstructure formed by TMA molecules adsorbed on a Au(111) surface. Distinct preferential orientations of the porous networks on Au(111) lead to the formation of peculiar TMA polymorphs that are stabilized only at the boundary between rotational molecular domains. Scanning tunneling microscopy (STM) and spectroscopy are used to investigate the electronic properties of both the molecular building blocks and the pores. Sub-molecular-resolution imaging and spatially resolved electronic spectroscopy reveal a remarkable change in the appearance of the molecules in the STM images at energies in the range of the lowest unoccupied molecular orbital, accompanied by highly extended molecular wave functions into the pores. The electronic structure of the pores reflects a weak confinement of surface electrons by the TMA network. Our experimental observations are corroborated by density-functional-theory-based calculations of the nanoporous structure adsorbed on Au(111)." @default.
• W2318631608 created "2016-06-24" @default.
• W2318631608 creator A5033455307 @default.
• W2318631608 creator A5039211990 @default.
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• W2318631608 date "2013-08-29" @default.
• W2318631608 modified "2023-10-14" @default.
• W2318631608 title "Probing the Electronic Properties of Trimesic Acid Nanoporous Networks on Au(111)" @default.
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• W2318631608 doi "https://doi.org/10.1021/la402282x" @default.
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• W2318631608 hasPublicationYear "2013" @default.
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