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- W2318672866 endingPage "4150" @default.
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- W2318672866 abstract "Mass-selected heteronuclear iron–copper carbonyl cluster anions CuFe(CO)n– (n = 4–7) are studied by infrared photodissociation spectroscopy in the carbonyl stretching frequency region in the gas phase. The cluster anions are produced via a laser vaporization supersonic cluster ion source. Their geometric structures are determined by comparison of the experimental spectra with those calculated by density functional theory. The experimentally observed CuFe(CO)n– (n = 4–7) cluster anions are characterized to have (OC)4Fe–Cu(CO)n−4 structures, each involving a C3v symmetry Fe(CO)4– building block. Bonding analysis indicates that the Fe–Cu bond in the CuFe(CO)n– (n = 4–7) cluster anions is a σ type single bond with the iron center possessing the most favored 18-electron configuration. The results provide important new insight into the structure and bonding of hetronuclear transition metal carbonyl cluster anions." @default.
- W2318672866 created "2016-06-24" @default.
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- W2318672866 date "2015-04-24" @default.
- W2318672866 modified "2023-09-25" @default.
- W2318672866 title "Infrared Photodissociation Spectroscopy of Mass-Selected Heteronuclear Iron–Copper Carbonyl Cluster Anions in the Gas Phase" @default.
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- W2318672866 doi "https://doi.org/10.1021/acs.jpca.5b02442" @default.
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