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- W2319099930 abstract "A series of monometallic Pt and Pd and alloyed Pt–Pd catalysts (mole ratio of Pt/Pd = 1, 4, and 0.25) were prepared with silica–alumina as support. CO chemisorption and X-ray diffraction (XRD) were applied to characterize the resulting samples. The performance of the catalysts for hydrodeoxygenation (HDO) for benzofuran (BF) was evaluated in a fixed-bed flow reactor at 280 °C and 3.0 MPa. Only one major route was found for the reaction network of HDO of BF among the catalysts. First, BF was transformed to 2,3-dihydrobenzofuran with the hydrogenation at the heterocyclic ring, followed by further conversion to octahydrobenzofuran at the benzene ring. The main hydrocarbon products are ethylcyclohexane and methylcyclohexane. The silica–alumina-supported catalysts also showed significant cracking activities, with the observation of the production of methylcyclohexane. The activity and product selectivity of Pt, Pd, and bimetallic Pt–Pd catalysts with the influence of the weight time were investigated in detail. Bimetallic Pt–Pd catalysts were higher in activity in the hydrogenation and the removal of oxygen from BF than their monometallic counterparts. The Pd4Pt1 catalyst presented the highest activity, with 99% conversion of BF and 100% selectivity toward 2,3-dihydrobenzofuran among all of the other catalysts at low weight time." @default.
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- W2319099930 date "2012-06-27" @default.
- W2319099930 modified "2023-09-23" @default.
- W2319099930 title "Hydrodeoxygenation of Benzofuran over Silica–Alumina-Supported Pt, Pd, and Pt–Pd Catalysts" @default.
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- W2319099930 doi "https://doi.org/10.1021/ef300694c" @default.
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