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• W2319326949 endingPage "4105" @default.
• W2319326949 startingPage "4102" @default.
• W2319326949 abstract "A bridged tetrahedryl-tetrahedrane (“TT”) was, theoretically, recognized as the holder of the chemical record for the shortest C–C single bond in a stable molecule. However, owing to its strained nature, this molecule is prone to rearrange to a carbene via ring contraction. Although TT was predicted to be stable to rearrangement at very low temperatures, our calculations find that, due to carbon quantum mechanical tunneling, even at 0 K it will immediately rearrange, with a half-life of only 4 ms. TT provides an excellent example of why tunneling effect should be considered in the stability analysis of a theoretically conceived molecule, even at cryogenic temperatures." @default.
• W2319326949 created "2016-06-24" @default.
• W2319326949 creator A5042210822 @default.
• W2319326949 date "2014-07-24" @default.
• W2319326949 modified "2023-10-18" @default.
• W2319326949 title "A Quantum Mechanical “Jack in the Box”: Rapid Rearrangement of a Tetrahedryl-Tetrahedrane via Heavy Atom Tunneling" @default.
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• W2319326949 doi "https://doi.org/10.1021/ol5017977" @default.
• W2319326949 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25058793" @default.
• W2319326949 hasPublicationYear "2014" @default.
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