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• W2319328623 endingPage "11285" @default.
• W2319328623 startingPage "11277" @default.
• W2319328623 abstract "There is a great interest in the utilization of silicon-based anodes for lithium-ion batteries. However, its poor cycling stability, which is caused by a dramatic volume change during lithium-ion intercalation, and intrinsic low electric conductivity hamper its industrial applications. A facile strategy is reported here to fabricate graphene oxide-immobilized NH2-terminated silicon nanoparticles (NPs) negative electrode (Si@NH2/GO) directed by hydrogen bonding and cross-linked interactions to enhance the capacity retention of the anode. The NH2-modified Si NPs first form strong hydrogen bonds and covalent bonds with GO. The Si@NH2/GO composite further forms hydrogen bonds and covalent bonds with sodium alginate, which acts as a binder, to yield a stable composite negative electrode. These two chemical cross-linked/hydrogen bonding interactions—one between NH2-modified Si NPs and GO, and another between the GO and sodium alginate—along with highly mechanically flexible graphene oxide, produced a robust network in the negative electrode system to stabilize the electrode during discharge and charge cycles. The as-prepared Si@NH2/GO electrode exhibits an outstanding capacity retention capability and good rate performance, delivering a reversible capacity of 1000 mAh g–1 after 400 cycles at a current of 420 mA g–1 with almost 100% capacity retention. The results indicated the importance of system-level strategy for fabricating stable electrodes with improved electrochemical performance." @default.
• W2319328623 created "2016-06-24" @default.
• W2319328623 creator A5019477992 @default.
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• W2319328623 date "2014-07-07" @default.
• W2319328623 modified "2023-10-13" @default.
• W2319328623 title "Graphene Oxide-Immobilized NH₂-Terminated Silicon Nanoparticles by Cross-Linked Interactions for Highly Stable Silicon Negative Electrodes" @default.
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• W2319328623 doi "https://doi.org/10.1021/am502597g" @default.
• W2319328623 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24922522" @default.
• W2319328623 hasPublicationYear "2014" @default.
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