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- W2319330772 abstract "We have observed the electron paramagnetic resonance (EPR) of ${mathrm{Gd}}^{3+}$ in both polycrystalline and single-crystal samples of dilute Pt: Gd alloys. The polycrystalline samples display a single resonance line whose thermal broadening is concentration dependent. Fully resolved fine structure appropriate to ${mathrm{Gd}}^{3+}$ in a cubic environment is obtained from the single-crystal samples. From these results a value for ${b}_{4}^{0}$ of +86 G is deduced, a value some three times larger than that found to date in any other cubic pure metals. It is shown conclusively that the experimental spectra from the single-crystal samples consist of the resolved single-ion fine-structure spectrum and an additional cluster line with the same $g$ value as the single-ion spectrum. For most directions in the {110} plane excellent agreement is obtained between the single-ion spectra and those simulated using the Barnes-Plefka motional-narrowing theory. The existence and behavior of the cluster line is qualitatively explained in terms of a cross-relaxation process. Finally it is shown that the excitation energy ${E}_{ifmmodepmelsetextpmfi{}}$ for the process $4{f}^{7}ensuremath{rightarrow}4{f}^{8}$ as involved in EPR is not the same as measured by optical experiments such as x-ray photoemission spectroscopy. A theory which describes this is capable of explaining the experimental exchange and crystal-field parameters." @default.
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- W2319330772 date "1980-09-01" @default.
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- W2319330772 title "Electron paramagnetic resonance of<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msup><mml:mrow><mml:mi mathvariant=normal>Gd</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn><mml:mo>+</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math>in platinum" @default.
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- W2319330772 doi "https://doi.org/10.1103/physrevb.22.2175" @default.
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