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- W2319481762 abstract "Abstract In the search for tricarbaporphyrinoids, a three‐component acid‐catalyzed condensation of azulene, 2,5‐bis[( p ‐tolyl)hydroxymethyl]thiophene, and an aryl aldehyde has been elaborated, affording the appropriate thiatriazuliporphyrinogens. The subsequent oxidation yielded a rare example of a macrocyclic organic tetracation, which can be readily and reversibly converted into macrocyclic tri‐ and dicarbocations by addition of one or two hydroxides bound at the meso position(s). Further insight into the influence of carbocation formation on the geometry, electronic structure, and magnetic manifestation in 1 H NMR spectroscopy has been obtained by using density functional theory calculations. The charge distribution was evaluated by mapping electron density surfaces with electrostatic potential (ESP)." @default.
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- W2319481762 date "2016-04-01" @default.
- W2319481762 modified "2023-10-05" @default.
- W2319481762 title "Carbocations Confined in a Thiatriazuliporphyrin Frame" @default.
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- W2319481762 doi "https://doi.org/10.1002/chem.201504752" @default.
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