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- W2320002971 abstract "Polymers that are capable of depolymerizing completely from head-to-tail upon cleavage of an end-cap from the terminus of the polymer have emerged recently as a new strategy for creating stimuli-responsive solid-state materials with amplified responses. In theory, solid-state materials made from these polymers will respond most efficiently to a stimulus in solution when the polymer end-caps are displayed into solution at the solid–liquid interface, rather than being buried in the solid-state material. This article defines two strategies for increasing the likelihood that end-caps are displayed at this interface. A microscale-pump made from films of depolymerizable poly(phthalaldehyde) serves as a test system for evaluating the location of end-caps in the films. By measuring the flow rate initiated by depolymerization of the polymers within the films, we determined that both the polymer length and hydrophilicity of the end-caps affect the density of end-caps at the solid–liquid interface." @default.
- W2320002971 created "2016-06-24" @default.
- W2320002971 creator A5001951940 @default.
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- W2320002971 date "2013-09-12" @default.
- W2320002971 modified "2023-10-15" @default.
- W2320002971 title "Accessibility of Responsive End-Caps in Films Composed of Stimuli-Responsive, Depolymerizable Poly(phthalaldehydes)" @default.
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- W2320002971 doi "https://doi.org/10.1021/ma401463e" @default.
- W2320002971 hasPublicationYear "2013" @default.
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