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• W2320167461 endingPage "1825" @default.
• W2320167461 startingPage "1820" @default.
• W2320167461 abstract "The diffusion and reaction are two general kinetic factors playing an important role in the structure development of materials. Upon diffusion limitation, a noncompact structure is easily formed, while a compact structure is usually formed in a reaction-limited condition. In this Article, we take the precipitation of calcium carbonate as an example to discover the roles of diffusion and reaction in shaping particles. By adjusting the diffusion and reaction in a three-cell reactor, we synthesize snow-shaped particles, which are a new morphology of calcium carbonate. The microscopic characterization shows that the microparticle is composed of aggregates of nanoparticles. Computer simulation suggests that the snow-shaped particle is formed in a condition that the diffusion and reaction compete to regulate the structure of particles and their compromise leads to the formation of snow-shaped morphology, which is confirmed by later experiments. The following discussion concentrates on the compromise concept to disclose its essence and role in shaping particles, which brings us a new view on the physical mechanisms governing the diversity of materials structures." @default.
• W2320167461 created "2016-06-24" @default.
• W2320167461 creator A5033211512 @default.
• W2320167461 creator A5082225017 @default.
• W2320167461 creator A5084854649 @default.
• W2320167461 date "2013-04-01" @default.
• W2320167461 modified "2023-10-16" @default.
• W2320167461 title "Dominant Role of Compromise between Diffusion and Reaction in the Formation of Snow-Shaped Vaterite" @default.
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• W2320167461 doi "https://doi.org/10.1021/cg301241s" @default.
• W2320167461 hasPublicationYear "2013" @default.
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