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- W2320259344 abstract "Time-resolved infrared absorption features in the 1800–2400 cm−1 region during a typical cycle in the oscillatory oxidation of CO over a platinum foil were obtained by Fourier transform infrared reflection absorption spectroscopy. Pretreatment of the foil in an oxidizing environment at high temperatures was found to be necessary to induce large-amplitude, stable oscillations. The oscillations are approximately square-wave in shape, with a high and a low reaction-rate branch. The level of chemisorbed CO in the high reaction-rate branch is typically below the noise level, while in the low reaction-rate branch substantial substantial surface coverages of CO can be observed. No evidence for CO bridge-bonded to the platinum substrate or chemisorbed in the presence of a subsurface Pt oxide could be found at any time during the oscillation cycle. Evidence is presented for the existence of CO islands in the low reaction-rate branch. It is also shown that the low reaction rate realized in this branch is not due to blocking of the surface by chemisorbed CO." @default.
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- W2320259344 date "1985-09-01" @default.
- W2320259344 modified "2023-09-24" @default.
- W2320259344 title "Studies on self-sustained reaction-rate oscillations" @default.
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- W2320259344 doi "https://doi.org/10.1016/0039-6028(85)91031-3" @default.
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