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• W2320365860 abstract "Using pump-probe spectroscopy, strong-field enhanced-ionization is found in an inner orbital of I${}_{2}$. A wave packet is launched in the $B$ state of I${}_{2}$, whose valence orbitals are ${ensuremath{sigma}}_{g}^{2}{ensuremath{pi}}_{u}^{4}{ensuremath{pi}}_{g}^{3}{ensuremath{sigma}}_{u}^{1}$, and singly ionized to the $text{I}+{text{I}}^{+}$ dissociation channel. The ionization signal peaks at two different internuclear separations: $ensuremath{sim}$7.3 and $ensuremath{sim}$8.7 a.u. The latter shows enhanced ionization of the ${ensuremath{sigma}}_{u}$ state which has been studied before with the ${{text{I}}_{2}}^{+}$ signal. However, the peak at smaller $R$ corresponds to enhanced ionization of the ${ensuremath{sigma}}_{g}$ state. The peak at $ensuremath{sim}$8.7 a.u. in the dissociating channel reveals that there could be strong mixing of different molecular orbitals when the two iodine atoms are pulled apart." @default.
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• W2320365860 date "2012-11-28" @default.
• W2320365860 modified "2023-09-27" @default.
• W2320365860 title "Enhanced ionization of an inner orbital of I2by strong laser fields" @default.
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• W2320365860 doi "https://doi.org/10.1103/physreva.86.051403" @default.
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