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• W2320426986 abstract "Hard x-ray photoemission studies of Ca${}_{3}$(Ru${}_{1ensuremath{-}x}$Ti${}_{x}$)${}_{2}$O${}_{7}$ with $x$ $=$ 0, 0.003, and 0.005 have been carried out to clarify the origin of the extremely high sensitivity of the metal-insulator (M-I) transition to the amount of Ti substitution. All the compounds show an antiferromagnetic transition followed by a structural transition at a temperature ${T}_{mathrm{S}}$, with decreasing temperature. For $x$ > 0, the structural transition is accompanied with a drastic M-I transition and the intensities of the screened peaks in the Ru 3$d$ core-level spectra are significantly reduced below ${T}_{mathrm{S}}$. The spectral weight of the valence band is concurrently shifted toward the higher binding energy side by an order of 2 eV, which shows that a strong electron correlation plays an essential role for the M-I transition at ${T}_{mathrm{S}}$ for $x$ > 0. These results provide strong evidence that Mott transition is induced by a minute amount of the Ti substitution in Ca${}_{3}$Ru${}_{2}$O${}_{7}$." @default.
• W2320426986 created "2016-06-24" @default.
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• W2320426986 date "2013-06-25" @default.
• W2320426986 modified "2023-10-01" @default.
• W2320426986 title "Mott transition extremely sensitive to impurities in Ca<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>3</mml:mn></mml:msub></mml:math>Ru<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>2</mml:mn></mml:msub></mml:math>O<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>7</mml:mn></mml:msub></mml:math>revealed by hard x-ray …" @default.
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• W2320426986 doi "https://doi.org/10.1103/physrevb.87.241107" @default.
• W2320426986 hasPublicationYear "2013" @default.
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