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• W2320771004 startingPage "8761" @default.
• W2320771004 abstract "A key factor controlling the interactions between surfaces in aqueous solutions is the surface charge density. Surfaces typically become charged though a titration process where surface groups can become ionized based on their dissociation constant and the pH of the solution. In this work, we use a Monte Carlo method to treat this process in a system with two planar surfaces with explicitly described ionizable sites in a salt solution. We focus on a system with a surface density of ionizable sites set to 4.8 nm–2, corresponding to silica. We find that the surface charge density changes as the surfaces come close to contact due to interactions between the ionizable groups on each surface. In addition, we observe an attraction between the surfaces above a threshold surface charge, in good agreement with previous theoretical predictions based on uniformly charged surfaces. However, close to contact we find the force is significantly different than for the uniformly charged case." @default.
• W2320771004 created "2016-06-24" @default.
• W2320771004 creator A5017862817 @default.
• W2320771004 creator A5053607565 @default.
• W2320771004 date "2011-06-14" @default.
• W2320771004 modified "2023-09-27" @default.
• W2320771004 title "Interactions Between Charged Surfaces with Ionizable Sites" @default.
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• W2320771004 doi "https://doi.org/10.1021/la201353u" @default.
• W2320771004 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21644585" @default.
• W2320771004 hasPublicationYear "2011" @default.
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