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- W2321117320 endingPage "1061" @default.
- W2321117320 startingPage "1056" @default.
- W2321117320 abstract "We have used visible-infrared sum-frequency generation spectroscopy to reveal fundamental characteristics of water structure at the fused silica surface. By studying a wide range of ionic strengths, from 0.05 mM to 4 M, we are able to comment on the contributions of second- and third-order nonlinearities to the spectroscopic response. Spectra obtained from extremely dilute salt concentrations provide evidence of the previously sought increasing surface charge with ionic strength. This is followed by a screening regime where the extent to which the surface field penetrates into the bulk is limited by the electrolyte. Data from intermediate salt concentrations reveal a few strongly ordered layers of water immediately adjacent to the surface. At high concentrations, we observe a significant disruption of solvent ordering. Together, the observation of these four distinct regimes provides a unified understanding of interfacial water structure in the presence of salt that consolidates previous reports in the literature." @default.
- W2321117320 created "2016-06-24" @default.
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- W2321117320 date "2011-04-15" @default.
- W2321117320 modified "2023-10-11" @default.
- W2321117320 title "The Effect of Salt on the Water Structure at a Charged Solid Surface: Differentiating Second- and Third-order Nonlinear Contributions" @default.
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- W2321117320 doi "https://doi.org/10.1021/jz200251h" @default.
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