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• W2321158022 abstract "We investigated the adsorbed states of 2,3,5,6-tetrafluoro-7,7,8,8-tetracyanoquinodimethane (F4-TCNQ) on Cu(100) using high-resolution electron energy loss spectroscopy (HREELS) and ultraviolet photoelectron spectroscopy (UPS). In the case of deposition at 90 K, the workfunction change increases up to ∼1.5 eV. In the case of deposition at 300 K, it saturates at ∼0.9 eV. In both cases, an occupied lowest unoccupied molecular orbital (LUMO) state of F4-TCNQ has been observed at 1.2 eV below the Fermi level. Both UPS and vibrational EELS results show that F4-TCNQ becomes an anion at 90 K. In addition, the extra weakening of C≡N bonds occurs at 300 K, involving the local interaction between the cyano groups in F4-TCNQ and surface Cu atoms, where the transformation into the rehybridized state is thermally activated. The bidirectional interaction including the donation from F4-TCNQ and the back-donation from Cu(100) can explain the difference in workfunction change." @default.
• W2321158022 created "2016-06-24" @default.
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• W2321158022 date "2010-09-20" @default.
• W2321158022 modified "2023-10-03" @default.
• W2321158022 title "Thermally Activated Transformation from a Charge-Transfer State to a Rehybridized State of Tetrafluoro-tetracyanoquinodimethane on Cu(100)" @default.
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• W2321158022 doi "https://doi.org/10.1021/jz100766k" @default.
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