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• W2321166768 abstract "The stability of gaseous vanadium molybdate and vanadium tungstates was confirmed by high-temperature mass spectrometry. A number of gas-phase reactions involving vanadium-containing salts were studied. On the basis of equilibrium constants, the standard formation enthalpies of gaseous VMoO4 (−676 ± 27 kJ/mol), VWO3 (−331 ± 29 kJ/mol), and VWO4 (−706 ± 23 kJ/mol) at 298 K were determined. A theoretical study of these salts revealed the structure with bidentate binding of the vanadium cation to the anion part to be the lowest-lying isomer, with a quartet spin state for VMoO4 and VWO4 molecules as well as a sextet spin state for the VWO3 molecule. On the basis of critical analysis of the literature data concerning standard formation enthalpies of gaseous VO and VO2, we adopted new values of ΔfH°(298) = 135 ± 10 kJ/mol for VO(g) and −185 ± 15.0 kJ/mol for VO2(g). Overall, the results obtained allowed us to estimate the standard formation enthalpy of VMoO3 to be −318 kJ/mol with an accuracy near 40 kJ/mol." @default.
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• W2321166768 date "2012-04-12" @default.
• W2321166768 modified "2023-09-25" @default.
• W2321166768 title "Gaseous Vanadium Molybdate and Tungstates: Thermodynamic Properties and Structures" @default.
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• W2321166768 doi "https://doi.org/10.1021/ic201644f" @default.
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