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• W2321305277 abstract "Abstract. Determining the processes which generate terrestrial carbonate deposits (tufas, travertines and associated chemical sediments) is a long-standing problem. Deposition of mineral products from solution reflects a complex combination of biological, equilibrium and kinetic processes, and the differences in products these processes produce are yet to be clearly demarked. Building on the groundbreaking work of previous authors, we propose that the underlying control on the processes leading to the deposition of these products can be most parsimoniously understood from the thermodynamic properties of their source solutions. Here, we report initial observations of the differences in product generated from spring and lake systems spanning a range of temperature : supersaturation space. We find that at high supersaturation, biological influences are masked by high rates of spontaneous nucleation and sedimentary products from these settings infrequently exhibit classic biomediated fabrics such as clotted micrite. Likewise, at high temperature exclusion of vascular plants and complex/diverse biofilms significantly inhibits the magnitude of biomediated precipitation, again impeding the likelihood of encountering the bio-type fabrics. Conversely, despite the clear division in product between extensive tufa facies associations and discontinuous deposits such as oncoid beds, no clear division can be identified between these systems in temperature : supersaturation space. We reiterate the conclusion of previous authors, which demonstrate that this division cannot be made on the basis of physico-chemical characteristics of the solution alone. We further provide a new case study of this division from two adjacent systems in the UK, where continuous tufa-like deposition is happening at a site with lower supersaturation than other sites exhibiting only discontinuous (oncoidal) deposition. However, a strong microbiological division is demonstrated between these sites on the basis of suspended bacterial cell distribution, which reach a prominent maximum where tufa-like deposits are forming. We conclude that at high supersaturation, the thermodynamic properties of solutions provide a highly satisfactory means of linking process and product, raising the opportunity of identifying water characteristics from sedimentological/petrological characteristics of ancient deposits. At low supersaturation, we recommend that future research focuses on geomicrobiological processes rather than the more traditional, inorganic solution chemistry approach dominant in the past." @default.
• W2321305277 created "2016-06-24" @default.
• W2321305277 creator A5024431903 @default.
• W2321305277 creator A5037106232 @default.
• W2321305277 creator A5082894907 @default.
• W2321305277 date "2013-09-11" @default.
• W2321305277 modified "2023-09-26" @default.
• W2321305277 title "Linking process and product in terrestrial carbonates using a solution thermodynamic approach" @default.
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• W2321305277 doi "https://doi.org/10.5194/esurfd-1-337-2013" @default.
• W2321305277 hasPublicationYear "2013" @default.
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