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- W2321314144 abstract "We report a new class of polymer electrolytes that exhibit high Li+-ionic conductivity and thermal stability up to 200 °C. The polymer electrolyte consists of a solvate ionic liquid ([Li(G4)][TFSA]), comprising an equimolar mixture of lithium bis(trifluoromethanesulfonyl)amide (Li[TFSA]) and tetraglyme (G4), and a well-defined ABA-triblock copolymer, polystyrene-b-poly(methyl methacrylate)-b-polystyrene (PSt-b-PMMA-b-PSt, SMS). The electrolyte is formed by the self-assembly of SMS, where the solvatophobic PSt segments serves as physical cross-linking points, and the solvatophilic PMMA segment with preferentially dissolved [Li(G4)][TFSA] forms ion-conduction paths. In the electrolyte, the preservation of the complex cation [Li(G4)]+ in the PMMA phase was demonstrated by pulsed-field gradient spin–echo (PGSE) NMR, Raman spectra, and thermogravimetric analysis. Because of the preservation of [Li(G4)]+, which hinders the direct interaction of Li+ with the polymer segment and the coupling of the ionic transport from the segmental motion, the room temperature ionic conductivity of the electrolyte reached an appreciable level (10–4–10–3 S cm–1)." @default.
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- W2321314144 date "2014-08-27" @default.
- W2321314144 modified "2023-10-17" @default.
- W2321314144 title "Gelation of Solvate Ionic Liquid by Self-Assembly of Block Copolymer and Characterization as Polymer Electrolyte" @default.
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- W2321314144 doi "https://doi.org/10.1021/ma501296m" @default.
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