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• W2321333942 abstract "The dynamics of electrons in image-potential resonances on the Ag(111) surface, i.e., image-potential states that are resonant with bulk bands, have been studied by time-resolved two-photon photoemission in combination with quantum-beat spectroscopy. Energies and lifetimes of these resonances were determined up to a quantum number $n=7$. Both quantities show a hydrogen-like scaling with quantum number $n$. The measured decay time of the first image-potential state ($n=1$), which is still located in the projected band gap, is 31.5(1.5) fs. The decay time decreases to 23(2) fs for the resonance $n=2$ and then increases up to 1 ps for $n=7$. It is concluded that the elastic decay of the resonances due to elastic electron transfer into the bulk is nearly one order of magnitude faster than the inelastic electron-hole pair decay. Nevertheless, the elastic decay is found to be slower than theoretically predicted. The pure dephasing times of the resonances $n=3$--7 are longer than the decay times. This suggests that electron-phonon scattering is weak despite a large bulk penetration of the resonance wave functions." @default.
• W2321333942 created "2016-06-24" @default.
• W2321333942 creator A5010448423 @default.
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• W2321333942 date "2011-12-07" @default.
• W2321333942 modified "2023-10-16" @default.
• W2321333942 title "Quantum-beat spectroscopy of image-potential resonances" @default.
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• W2321333942 doi "https://doi.org/10.1103/physrevb.84.245402" @default.
• W2321333942 hasPublicationYear "2011" @default.
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