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- W2321348000 endingPage "4758" @default.
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- W2321348000 abstract "The syntheses as well as detailed studies on the thermal, photophysical, and self-organization properties of a new series of phosphole-based ladder-type materials with exocyclic 5-alkylthienyl substituents are reported. The studies also include DFT calculations that provide support for the experimentally determined photophysics. In contrast to the related “phosphole-lipids” with fused conjugated head that exhibit low luminescence in solution but high luminescence in the solid state, the new system is highly luminescent in both solution and the solid state. The extensive structure–property study reported herein revealed that the physical properties of the new species can significantly be tuned via the size of the conjugated system of the head group, the functionalization of the phosphorus center, as well as the length of the thiophene-appended alkyl chain that impacts the intermolecular interactions via π–π stacking, ionic, and van der Waals interactions, respectively. This molecular engineering approach allows to access materials with intriguing properties that range from highly emissive oils to self-organized one-dimensional fibers." @default.
- W2321348000 created "2016-06-24" @default.
- W2321348000 creator A5023565096 @default.
- W2321348000 creator A5036580395 @default.
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- W2321348000 date "2013-02-27" @default.
- W2321348000 modified "2023-10-07" @default.
- W2321348000 title "Molecular Engineering of the Physical Properties of Highly Luminescent π-Conjugated Phospholes" @default.
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- W2321348000 doi "https://doi.org/10.1021/jp3115012" @default.
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