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• W2321370356 abstract "Molecular high-order-harmonic generation and molecular-orbital ionization rates are calculated for the CO, ${text{H}}_{2}text{CO}$, ${text{CO}}^{+}$, and ${text{H}}_{2}{text{CO}}^{+}$ molecules using numerical solutions of Kohn-Sham equations of time-dependent density-functional theory in the nonlinear nonperturbative regime of laser-molecule interactions. Different laser-molecule orientations (ensuremath{theta} = 0, 90ifmmode^circelsetextdegreefi{}, and 180ifmmode^circelsetextdegreefi{}) and intensities (8.7 ifmmodetimeselsetexttimesfi{} 10${}^{13}$, 3.5 ifmmodetimeselsetexttimesfi{} 10${}^{14}$, and 1.4 ifmmodetimeselsetexttimesfi{} 10${}^{15}$ W/cm${}^{2}$) are used. Results show that at wavelength ensuremath{lambda} = 800 nm, the ionization rate maxima are influenced for each molecular orbital by the interplay between its ionization potential, its geometrical shape, and the laser polarization axis. Molecular high-order-harmonic generation is further studied by a time profile analysis and a time-dependent electron localization function. A comparison of the data between CO and ${text{H}}_{2}text{CO}$ illustrates the importance of the protons on the electron distributions, ionization, and recollision dynamics in intense fields." @default.
• W2321370356 created "2016-06-24" @default.
• W2321370356 creator A5007962222 @default.
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• W2321370356 date "2014-02-12" @default.
• W2321370356 modified "2023-09-27" @default.
• W2321370356 title "Ionization and harmonic generation in CO and<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mtext>H</mml:mtext><mml:mn>2</mml:mn></mml:msub><mml:mtext>CO</mml:mtext></mml:math>and their cations with ultrashort intense laser pulses with time-dependent density-functional theory" @default.
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• W2321370356 doi "https://doi.org/10.1103/physreva.89.023414" @default.
• W2321370356 hasPublicationYear "2014" @default.
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