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- W2321497052 abstract "A fundamental Poisson-Nernst-Planck-Stokes model is presented for the impedance response of a long nanochannel under zero bias, capturing the effects of surface conduction and the coupling between transverse momentum and axial ion distribution in a manner reminiscent of Taylor dispersion. This is shown to result in a shift of the impedance frequency spectrum with bulk concentration similar to previous experimental observation [Schiffbauer, Liel, and Yossifon, Phys. Rev. E 89, 033017 (2014)]. It further predicts an additional downward shift in frequency with increasing viscosity. Finally, the introduction of a phenomenological model for the impedance response of a dynamic Stern layer in parallel with the diffuse layer transport model is shown to yield good agreement between theory and experiment. As a result, we are able to obtain an equivalent circuit model based on the fundamental model and proposed corrections." @default.
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- W2321497052 date "2014-05-19" @default.
- W2321497052 modified "2023-09-25" @default.
- W2321497052 title "Influence of electric-double-layer structure on the transient response of nanochannels" @default.
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- W2321497052 doi "https://doi.org/10.1103/physreve.89.053015" @default.
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