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- W2321736300 abstract "We have investigated the frequency-dependent interfacial electrical properties of nanocrystalline diamond films that were covalently linked to DNA oligonucleotides and how these properties are changed upon exposure to complementary and noncomplementary DNA oligonucleotides. Frequency-dependent electrical measurements at the open-circuit potential show significant changes in impedance at frequencies of >10(4) Hz when DNA-modified diamond films are exposed to complementary DNA, with only minimal changes when exposed to noncomplementary DNA molecules. Measurements as a function of potential show that at 10(5) Hz, the impedance is dominated by the space-charge region of the diamond film. DNA molecules hybridizing at the interface induce a field effect in the diamond space-charge layer, altering the impedance of the diamond film. By identifying a range of impedances where the impedance is dominated by the diamond space-charge layer, we show that it possible to directly observe DNA hybridization, in real time and without additional labels, via simple measurement of the interfacial impedance." @default.
- W2321736300 created "2016-06-24" @default.
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- W2321736300 date "2004-07-10" @default.
- W2321736300 modified "2023-10-14" @default.
- W2321736300 title "Interfacial Electrical Properties of DNA-Modified Diamond Thin Films: Intrinsic Response and Hybridization-Induced Field Effects" @default.
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- W2321736300 doi "https://doi.org/10.1021/la036460y" @default.
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