FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2321811866> ?p ?o ?g. }

• W2321811866 endingPage "7603" @default.
• W2321811866 startingPage "7590" @default.
• W2321811866 abstract "In organic materials, exciton dissociation into free charges requires overcoming an electron–hole Coulomb interaction that exceeds the thermal energy and may still be large after charge transfer at a donor/acceptor interface. We analyze the factors affecting efficiency of charge separation and subsequent removal of electrons and holes from such a donor–acceptor interface and suggest strategies for optimizing these processes. Energy transfer, charge separation, and charge transfer in the vicinity of the donor–acceptor interface are studied within a common theoretical framework based on a quantum master equation, for a model system with realistic excitation energies and electronic couplings. We find that enhancing the efficiency of both charge transfer from the donor to the acceptor and of charge removal from the donor–acceptor interface requires an intricate balance between the extent of electronic delocalization throughout the material and rates of energy dissipation. For very large exciton binding energies, cascade charge separation in systems with more than one donor and one acceptor species, such as molecular polyads, is found to greatly facilitate the dissociation of geminate pairs. Our calculations predict charge separation on subpicosecond timescales for several parameter combinations, leading to design principles for enhancing charge separation in multichromophore systems." @default.
• W2321811866 created "2016-06-24" @default.
• W2321811866 creator A5019265176 @default.
• W2321811866 creator A5035885969 @default.
• W2321811866 creator A5050599213 @default.
• W2321811866 creator A5069119629 @default.
• W2321811866 date "2015-03-30" @default.
• W2321811866 modified "2023-09-23" @default.
• W2321811866 title "Coherent and Incoherent Contributions to Charge Separation in Multichromophore Systems" @default.
• W2321811866 cites W1584656301 @default.
• W2321811866 cites W1649271673 @default.
• W2321811866 cites W181097001 @default.
• W2321811866 cites W1964835060 @default.
• W2321811866 cites W1966423034 @default.
• W2321811866 cites W1968295437 @default.
• W2321811866 cites W1975134990 @default.
• W2321811866 cites W1975534595 @default.
• W2321811866 cites W1981717389 @default.
• W2321811866 cites W1991243452 @default.
• W2321811866 cites W2001128599 @default.
• W2321811866 cites W2005144366 @default.
• W2321811866 cites W2005355378 @default.
• W2321811866 cites W2013765201 @default.
• W2321811866 cites W2014266475 @default.
• W2321811866 cites W2015683881 @default.
• W2321811866 cites W2016564617 @default.
• W2321811866 cites W2017841399 @default.
• W2321811866 cites W2021416051 @default.
• W2321811866 cites W2023392376 @default.
• W2321811866 cites W2031200233 @default.
• W2321811866 cites W2034771628 @default.
• W2321811866 cites W2037773093 @default.
• W2321811866 cites W2041363197 @default.
• W2321811866 cites W2049745418 @default.
• W2321811866 cites W2051432425 @default.
• W2321811866 cites W2055855475 @default.
• W2321811866 cites W2064076038 @default.
• W2321811866 cites W2066881078 @default.
• W2321811866 cites W2068906400 @default.
• W2321811866 cites W2069457460 @default.
• W2321811866 cites W2071837783 @default.
• W2321811866 cites W2072350015 @default.
• W2321811866 cites W2072396741 @default.
• W2321811866 cites W2078526451 @default.
• W2321811866 cites W2080879353 @default.
• W2321811866 cites W2081232414 @default.
• W2321811866 cites W2082308188 @default.
• W2321811866 cites W2085123660 @default.
• W2321811866 cites W2092063744 @default.
• W2321811866 cites W2095668864 @default.
• W2321811866 cites W2096320304 @default.
• W2321811866 cites W2097795991 @default.
• W2321811866 cites W2097804096 @default.
• W2321811866 cites W2098527861 @default.
• W2321811866 cites W2100077118 @default.
• W2321811866 cites W2100707163 @default.
• W2321811866 cites W2108044367 @default.
• W2321811866 cites W2122047873 @default.
• W2321811866 cites W2127296814 @default.
• W2321811866 cites W2130297415 @default.
• W2321811866 cites W2131873809 @default.
• W2321811866 cites W2145252402 @default.
• W2321811866 cites W2150397710 @default.
• W2321811866 cites W2159816551 @default.
• W2321811866 cites W2166109017 @default.
• W2321811866 cites W2167346196 @default.
• W2321811866 cites W2172154891 @default.
• W2321811866 cites W2174056229 @default.
• W2321811866 cites W2312307123 @default.
• W2321811866 cites W2318020837 @default.
• W2321811866 cites W2322476271 @default.
• W2321811866 cites W2324252347 @default.
• W2321811866 cites W2324640297 @default.
• W2321811866 cites W2330348192 @default.
• W2321811866 cites W2334938935 @default.
• W2321811866 cites W2488661712 @default.
• W2321811866 cites W2951888557 @default.
• W2321811866 cites W3100505277 @default.
• W2321811866 cites W4213245659 @default.
• W2321811866 cites W4246222558 @default.
• W2321811866 cites W4299788320 @default.
• W2321811866 doi "https://doi.org/10.1021/jp5127859" @default.
• W2321811866 hasPublicationYear "2015" @default.
• W2321811866 type Work @default.
• W2321811866 sameAs 2321811866 @default.
• W2321811866 citedByCount "19" @default.
• W2321811866 countsByYear W23218118662015 @default.
• W2321811866 countsByYear W23218118662017 @default.
• W2321811866 countsByYear W23218118662018 @default.
• W2321811866 countsByYear W23218118662019 @default.
• W2321811866 countsByYear W23218118662020 @default.
• W2321811866 countsByYear W23218118662021 @default.
• W2321811866 countsByYear W23218118662022 @default.
• W2321811866 crossrefType "journal-article" @default.
• W2321811866 hasAuthorship W2321811866A5019265176 @default.
• W2321811866 hasAuthorship W2321811866A5035885969 @default.
• W2321811866 hasAuthorship W2321811866A5050599213 @default.
• W2321811866 hasAuthorship W2321811866A5069119629 @default.

• next