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• W2321875767 startingPage "2174" @default.
• W2321875767 abstract "Reactions between [Rh2(CH3COO)4] with 2,6-diaminopurine (HDap) or 6-chloro-2-aminopurine (HClap) and [Rh2((CH3)3CCOO)4] with HClap produce, three new dirhodium(II) carboxylate complexes of the general form, [Rh2(RCOO)4(Purine)2] (R= CH3, (CH3)3C). Single crystal X-ray diffraction studies confirm that in all cases the purine coordinates to the axial position of the dirhodium(II)tetracarboxylate unit. However, while the complex obtained with HDap features the typical purine binding mode via N(7), complexes containing HClap show unusual N3 coordination. This is an extremely rare instance of an unrestricted purine binding via N3. Some rationalization of these data is offered based on a series of DFT calculations." @default.
• W2321875767 created "2016-06-24" @default.
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• W2321875767 date "2013-02-01" @default.
• W2321875767 modified "2023-10-18" @default.
• W2321875767 title "Substituent and Noncovalent Interaction Effects in the Reactivity of Purine Derivatives with Tetracarboxylato-dirhodium(II) Units. Rationalization of a Rare Binding Mode via N3" @default.
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• W2321875767 doi "https://doi.org/10.1021/ic302602c" @default.
• W2321875767 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23373427" @default.
• W2321875767 hasPublicationYear "2013" @default.
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