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- W2322126114 abstract "An efficient, step-economical, and scalable approach to the synthesis of polypropionate stereotriads has been developed. Either 2-butyne or propyne is subjected to rhodium-catalyzed silylformylation and in situ crotylation of the resulting aldehydes. Tamao oxidation under either “standard” conditions or “aprotic” conditions then delivers the completed stereotriads in a three-step, two-pot sequence. In contrast to the classical Roche ester approach, the α-stereocenter is obtained for “free.”" @default.
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- W2322126114 date "2014-02-06" @default.
- W2322126114 modified "2023-09-25" @default.
- W2322126114 title "Beyond the Roche Ester: A New Approach to Polypropionate Stereotriad Synthesis" @default.
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- W2322126114 doi "https://doi.org/10.1021/ol500051e" @default.
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