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- W2322387516 abstract "A simple methodology is employed to demonstrate the manifestation of energy quantization in classical, steady-state nucleation of small, geometrically precise clusters. With the use of recent dispersive kinetic theory outcomes, fresh insights into nonsteady-state nucleation-and-growth processes are also put forth. The impetus for this work stems from the fact that classical nucleation theory (CNT), which is often a poor predictor of nucleation rates, relies on macroscopic, continuous material properties to describe the physicochemical characteristics of the critical nucleus that, in turn, determines the activation energy barrier for nucleation; those quantities are not physically relevant on the atomic/nanometer scale. While it is shown that the low apparent interfacial tension of the smallest critical clusters likely gives rise to a very diffuse interface, their crystalline core provides a natural high-energy (metastable) state useful in determining the activation energy. For simplicity, it is assumed th..." @default.
- W2322387516 created "2016-06-24" @default.
- W2322387516 creator A5042818980 @default.
- W2322387516 date "2013-03-26" @default.
- W2322387516 modified "2023-09-27" @default.
- W2322387516 title "Atomistic Description of Two-Dimensional Hexagonal Close-Packed Critical Nuclei Exhibiting Quantization of the Activation Energy Barrier" @default.
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- W2322387516 doi "https://doi.org/10.1021/cg400020v" @default.
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